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Magnetic Structures in Ucusn Article Review

Review by : aguspur
Visits : 13  words: 300   Published: May 16, 2008
UCuSn was thought to crystallize in the CaIn2-type structure.  It orders antiferromagnetically at T=60K and exhibits a moderately enhanced linear heat capacity coefficient (53mJ/molK2).  A second anomaly visible in all bulk properties around 30K was interpreted in terms of a drastic change in the Fermi surface with no magnetic phase transition.  Further work reported that UCuSn crystallizes in a structure closely related to the hexagonal GaGeLi structure namely the orthorhombic P21cn.  Soon after that, Szytula et al. claimed that the structure should be P63mc while P21cn should be disregarded.  Nevertheless, they indicated not being able to fit all peaks assuming the hexagonal symmetry.  This paper reports neutron-diffraction results on UCuSn indicating that the compound undergoes two magnetic transitions around TN=62K and TM=25K. At T=52K, UCuSn exhibits a noncollinear arrangement of uranium moments of 1.5 Bohr-magneton/U-atom with components in all three principal direction and crystallizing in P21cn structure.



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